General Shape Control of Colloidal CdS, CdSe, CdTe Quantum Rods and Quantum Rod

General Shape Control of Colloidal CdS,CdSe,CdTe Quantum Rods and Quantum Rod Heterostructures

Felice Shieh,?Aaron E.Saunders,?and Brian A.Korgel*

Department of Chemical Engineering,Texas Materials Institute,Center for Nano-and Molecular Science and Technology,Uni V ersity of Texas,Austin,Texas 78712Recei V ed:February 21,2005;In Final Form:March 25,2005

We report a general synthetic method for the formation of shape-controlled CdS,CdSe and CdTe nanocrystals and mixed-semiconductor heterostructures.The crystal growth kinetics can be manipulated by changing the injection rate of the chalcogen precursor,allowing the particle shape s spherical or rodlike s to be tuned without changing the underlying chemistry.A single injection of precursor leads to isotropic spherical growth,whereas multiple injections promote epitaxial growth along the length of the c -axis.This method was extended to produce linear type I and type II semiconductor nanocrystal heterostructures.

The ability to rationally tune the shape of colloidal nano-crystals from spheres to rods has been actively sought during the last several years and several approaches have been developed,including metal particle-induced formation of semi-conductor nanorods and nanowires by “VLS”growth,1-4spontaneous nanocrystal assembly into wires 5,6and template-directed nanowire/nanorod formation,7,8which have been ap-plied to a wide range of materials,including group II -VI,III -V and IV semiconductors.Colloidal nanorods of semiconductors and metals have also been synthesized in coordinating solvents by manipulating the capping ligands,the ligand-solvent pair,reactant concentration,or the synthesis temperature.9-15In most colloidal approaches that do not rely on a metal seed particle or a template to direct growth,there is limited fundamental understanding of how to control nanorod formation.Here,we demonstrate general synthetic shape control of CdE (E:S,Se,Te)nanocrystals in coordinating solvents by sequential chalcogenide precursor injection.This very simple approach separates an initial particle nucleation event,followed by selective kinetically controlled epitaxial growth of the hexagonal {002}planes to generate rods.The rod length is determined by the number of injections.We further demonstrate the generality of this method by producing nanorod heterostructures of CdS/CdTe/CdS and CdTe/CdSe/CdTe.

The standard arrested precipitation procedure for colloidal nanocrystals such as CdSe utilizes the injection of organome-tallic precursors into a hot coordinating solvent,such as a mixture of trioctylphosphine (TOP)and trioctylphosphine oxide (TOPO).16This method gives a burst of particle nucleation followed by slow growth.In most cases,spherical particles are produced,and the temporal separation between nucleation and growth helps to achieve relatively narrow size distributions.In some exceptional cases,rod-shaped particles form and can be isolated,as first demonstrated by Peng,Alivisatos and co-workers for CdSe.9CdSe has a hexagonal crystal structure

(wurtzite),and it is now well-established that some growth conditions favor crystallization in the ?002?direction.17Here we show a general method for promoting rod growth of CdS,CdSe and CdTe nanocrystals that does not rely on changing the underlying reaction chemistry.Simply by injecting the chalcogenide precursor in a stepwise manner,selective epitaxial deposition on the {002}surface can be promoted to elongate the initial nuclei into nanorods.This kinetic control of the nanocrystal shape is readily applied to the Cd chalcogenides and we have extended this approach to make nanorod hetero-structures (Figure 1).

Figure 2shows CdS,CdSe and CdTe nanocrystals and nanorods produced using a modification of Peng’s procedure for CdE nanocrystals.18Both nanocrystals and nanorods are produced using the same chemistry,by first loading the reaction flask with Cd precursor solution and then adding a stoichiometric amount of chalcogen precursor.Nanorods are produced by introducing the chalcogen precursor in multiple sequential injections as opposed to a single injection.Briefly,CdO is heated in a mixture of n -tetradecylphosphonic acid (TDPA)and trioctylphosphine oxide (TOPO)to form a starting solution with a Cd-TDPA complex as the Cd source.Separately,S,Se,or Te,is dissolved in trioctylphosphine (TOP),and then added as the chalcogen source to the reaction.The chalcogen-TOP solution is injected into the optically clear Cd-TDPA/TOPO mixture at ～300°C in either a batch single injection or multiple injection procedure to produce either spherical or rodlike particles [see Supporting Information for details].

In Figure 2,the CdTe nanorods are 30.7(6.3nm long with an average aspect ratio of 6,the CdS nanorods are 26.4(9.1nm with an aspect ratio of 8,and the CdSe nanorods are 12.6( 2.3nm long with an average aspect ratio of 3.The nanocrystals exhibit the wurtzite crystal structure with the nanorods elongated in the ?002?https://www.sodocs.net/doc/d82470341.html,parison of X-ray diffraction (XRD)patterns for nanorods and nanocrystals such as those in Figure 3for CdTe reveals that the nanorods exhibit a more intense and narrower (002)peak relative to the spheres due to their difference in shape.After deconvoluting the (100),*Corresponding author.Tel:512-471-5633.Fax:512-471-7060.E-mail:korgel@https://www.sodocs.net/doc/d82470341.html,.

?These authors contributed equally to this work.8538

2005,109,8538-

8542Published on Web 04/12/2005

10.1021/jp0509008CCC:$30.25

?2005American Chemical Society

(002)and (101)peaks for the CdTe nanorods in Figure 3,the Scherrer equation gives a rod length and diameter of 30and 5nm,in agreement with TEM images.In contrast to the rods,the spherical particles exhibit several diffraction peaks with reduced intensity (particularly the (100),(101)and (103)peaks),giving the superficial appearance of the zinc blende (cubic)crystal structure.This peak attenuation results from the signifi-cant number of stacking faults in the ?002?direction,as has been observed previously for CdSe nanocrystals.16From our TEM images of nanocrystals and nanorods,spherical particles have a significant number of twinning and stacking faults,whereas the nanorods do not.However,more data are still needed to verify this difference in defect density,as stacking faults of the type observed from the spherical nanocrystal in Figure 2g can only be observed from rods with the beam oriented in the ?110?direction.

The evolution of particle size and shape was followed by periodically withdrawing ～0.5mL aliquots from the reaction.Figure 3shows CdTe nanorods at different stages in the multiple precursor injection process.Early in the reaction,after two injections of Te-TOP,short nanorods s “nanorice”s form (Figure 3a).As more precursor is injected,the nanorods grow axially without an increase in diameter.The nanorods elongate until the TDPA-complexed Cd precursor is depleted.Depletion of the Cd-TDPA complex and further heating results in the subsequent ripening of the nanorods and they reshape into

spherical particles (Figure 3c,d).The nanorods can be isolated by quenching the reaction immediately after the final chalco-genide precursor injection.We have not observed rod to sphere ripening of nanorod dispersions at room temperature,with dispersions that have been stable for months.

UV -visible absorbance and photoluminescence (PL)spectra provide a useful metric to follow the nanocrystal shape evolution from spheres to rods.Figure 3e shows representative data for CdTe nanorods.The relatively sharp exciton peak and the appearance of higher order features in the absorbance spectra indicate that the samples are relatively size-and shape-monodisperse.Furthermore,the optical properties are good,with band edge PL and narrow peak widths.The most important aspect of the optical data is the gradually increasing Stokes shift as the aspect ratio of the rods increases,which is consistent with expectations for nanorods.9,19,20In general,the quantum yield (QY)of the nanocrystals decreases slightly throughout the reaction and does not appear to directly correlate with particle shape.The initial aliquot,after a single injection,had a QY of 1.7%when compared to Rho6G and slowly decreased to less than a percent by the end of the reaction.After the final

Figure 1.Semiconductor nanorod and heterostructure growth.Multiple injections of a chalcogenide precursor (brown atoms)into a growth solution of cadmium (white atoms)promotes growth along the ?001?direction and forms semiconductor nanorods.Addition of a second chalcogenide source (green atoms)forms rod ends of a second composition,allowing for the synthesis of nanorod semiconductor heterostructures with tunable properties.

Figure 2.TEM images of CdS,CdSe,and CdTe nanocrystals.The images on the left show spheres produced by single injection and the right correspond to rods formed upon multiple precursor injection for (a,b)CdTe;(c,d)CdSe;and (e,f)CdS.Spherical nanocrystals,such the CdTe nanocrystal in (g),show a high occurrence of stacking faults;whereas,the nanorods (h)do not.The nanorods grow in the ?002?direction,as shown in (h).

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precursor injection,the particles continue to increase in size and the absorbance spectra further red shift;however,the Stokes shift decreases,consistent with a shape evolution back to spheres.

To further prove the generality of the sequential injection method for CdS,CdSe and CdTe nanorods,we prepared nanorod “heterostructures”consisting of a nanorod core of one material sandwiched between two ends of a different material.Nanorods of CdTe for example,were first synthesized,and then elongated with a different material,such as CdSe or CdS,through multiple injections of a second chalcogenide precursor.In this way,heterostructures with either type I (CdS/CdTe/CdS)or type II (CdTe/CdSe/CdTe)band offsets were generated.Figure 4shows TEM and dark field scanning transmission electron microscopy (STEM)images of the nanorod heterostructures generated by sequential injection.

CdTe/CdSe/CdTe heterostructure nanorods are grown by forming CdSe nanorods (Figure 4a)from multiple injections of Se-TOP followed by sequential injections of Te-TOP.The addition of Te-TOP promotes the epitaxial growth of CdTe at the ends of the CdSe nanorods (Figure 4b).The nanorods appear to elongate without any change in particle diameter.Nanorod growth occurs exclusively at the reactive {002}planes at the rod ends.The optical properties of the heterojunction nanorods were also followed during the growth process.Several distinctive features help confirm that heterojunction nanorods are evolving,as opposed to the formation of core/shell particles or the nucleation of additional particles,discussed below.

For CdTe/CdSe/CdTe nanorods,the PL intensity quenches upon the addition of the CdTe end caps (Figure 5c)and the QY drops more than an order of magnitude after the first injection of Te-TOP,from 0.24%to 0.01%,and remains essentially unchanged after further Te-TOP injections.Figure 6shows the room-temperature PL spectra for these heterostruc-ture nanorods as a function of increased end cap length.The two peaks in the spectra result from electron -hole recom-bination in the CdSe nanorod core (band edge peak)and at the

CdSe/CdTe interface (long wavelength peak).15,21-23Due to the staggered type II band offset,there is an energy barrier preventing electron transfer from the CdSe core into the CdTe ends,whereas hole transfer from the CdSe core into the CdTe ends is energetically downhill.As the end caps lengthen,the relative likelihood of electron -hole recombination at the CdSe/CdTe interface increases,leading to decreased PL QY.15PL quenching is consistent with CdTe addition to the surface

Figure 3.Evolution in size and shape of CdTe nanorods.After two sequential injections,low aspect ratio nanorods form,as in (a).(b)Further sequential injections elongate the nanorods to achieve aspect ratios greater than 10.Upon further heating,the rods undergo a shape transition to spheres,initially increasing in diameter with decreasing length (c)and ultimately reshaping into spheres (d).(e)Absorbance and PL of CdTe nanocrystal aliquots taken during rod growth (λexc )560nm);the Stokes shift increases as the rods lengthen,then decreases as ripening occurs.(f)XRD patterns of CdTe nanorods and nanocrystals indexed to the wurtzite crystal structure.

Figure 4.CdTe/CdSe/CdTe (type II)and CdS/CdTe/CdS (type I)heterojunction nanorods.(a)TEM images of CdSe nanorod cores.TEM images of heterojunction nanorods after depositing CdTe at the ends of the CdSe nanorods (b)before and (c)after the CdTe caps ripen into spheres.(d)TEM and (e)dark-field STEM image CdTe/CdSe/CdTe nanorods after the CdTe end caps have ripened into spheres,giving the bar bell shape.(f)CdTe nanorods used to template CdS end caps.(g,h)TEM images of CdS/CdTe/CdS nanorods.

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of the existing CdSe nanocrystals and is not consistent with the nucleation and growth of separate CdTe nanocrystals(TEM also confirms that nucleation and growth of new particles does not occur).The observation of PL quenching is,in itself,not sufficient to confirm that CdTe is adding to the end caps,as core/shell deposition could also give rise to PL quenching.How-ever,core/shell deposition of the smaller band gap semiconduc-tor,CdTe,is expected to shift the absorption edge to longer wavelength,21,22which is not observed(Figure5a).For rods longer than the Bohr exciton diameter,but thinner than the Bohr exciton diameter,the nanorod diameter is solely responsible for energy level quantization and the size-dependent shift in the optical spectra.9,24The fact that the absorbance spectra do not noticeably shift to longer wavelengths with increasing amounts of CdTe deposition indicates that CdTe deposits selectively at the{002}end cap faces of the CdSe nanorods.

One thing to note about the CdTe/CdSe/CdTe nanorods is that at long reaction times,the nanorods ripen into spherical CdSeTe alloyed nanocrystals.The CdTe end caps first“ball up”to form dumbbell structures that eventually ripen into spheres.An example of such a dumbbell structure is shown in Figure4.The compositional variation along the length of the rod is especially apparent in the dark field scanning transmission electron microscopy(STEM)image taken using a high angle annular dark field(HAADF)detector(Figure4e).This“Z-contrast”image shows the lighter CdTe isolated in the dumbbell ends and the darker CdSe in the nanorod core.As the nanorod continues to ripen in the hot reaction environment,the absor-bance spectra flattens and the absorption edge shifts far into the near-IR as the rods reshape into alloyed spherical particles. The optical properties of the CdS/CdTe/CdS nanorods are also consistent with heterostructure nanorod formation with sequential precursor injection.In this case,the addition of CdS enhances the PL intensity of the CdTe nanorods(Figure5d). The QY increases an order of magnitude from0.37%for bare initial CdTe rods to1.70%as additional CdS is epitaxially added.If the mixture is slowly cooled to room temperature, allowing the sulfur caps additional time to grow and allowing interfacial and surface defects to anneal enhanced the PL(Figure 5d)for QY values reaching as high as20%.There is no sign of additional PL from separate CdS nanocrystals.The absorbance spectra in Figure5b are again,consistent with nanorod forma-tion,with the absorption edge staying fixed at one wavelength with the addition of the CdS.Core/shell particles would also be expected to exhibit these kind of changes in the optical properties;12however,the TEM images show that the rods are getting longer with additional S-TOP injections,confirming that CdS is growing epitaxially at the ends of the nanorods.In contrast to the CdTe/CdSe/CdTe nanorods,the CdS/CdTe/CdS nanorods do not undergo ripening at long reaction times,which is qualitatively different than what occurs for the CdTe nanorods. Our ability to extend the sequential injection approach to nanorod heterostructures is in fact not that surprising for CdE nanocrystals,as surface reaction controlled growth of CdE-based nanorod heterostructures has been observed in a couple of recent instances.For example,Alivisatos and co-workers found that CdSe/CdS/CdSe rods and CdTe tetrapods(on CdSe seed particles)formed in certain cases when they attempted to make core/shell nanocrystals.15Weller and co-workers found some-what similar epitaxial interfacing between CdSe core particles and CdS rodlike extensions.13Also,Banin’s group25recently demonstrated the selective deposition of gold tips at the ends

Figure5.Optical properties of CdTe/CdSe/CdTe and CdS/CdTe/CdS heterojunction nanorods.(a)Absorbance spectra for CdTe/CdSe/CdTe heterojunction rods with multiple chalcogen precursor injections;at long reaction times,ripening increases the particle size past the Bohr diameter,giving the appearance of bulk material at long times.PL is not reported as it is quenched due to the type II band offset.(b) Absorbance and PL of CdS/CdTe/CdS heterostructure nanorods.(c,d) PL peak intensity as a function of precursor injections.The type II band offset of CdTe/CdSe/CdTe results in quenching,whereas the type I band offset CdS/CdTe/CdS increases the PL quantum yield.(λexc )550nm for CdTe/CdSe/CdTe at550nm;andλ

exc

)610nm for CdS/CdTe/CdS).Figure6.Room temperature photoluminescence of CdTe/CdSe/CdTe heterostructure quantum rods.The PL of the CdSe nanorods is shown in(a)and exhibits only band edge emission.A broad peak centered at approximately800nm appears and increases in intensity after one(b), two(c)and three(d)injections of Te into the reaction,indicative of type II recombination.The PL intensity is quenched with increasing Te injections;the scale shows the relative intensity normalized to the original CdSe sample.

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of CdSe nanorods and Kudera et al.26demonstrated selective PbSe deposition on the tips of CdS and CdSe nanorods s providing further indication that the wurtzite CdE{002}surface is the most reactive.We simply demonstrate here the general capability to epitaxially elongate CdE nanorods using sequential injection of precursor.By changing the composition of the precursor,the composition of the end cap can be manipulated, allowing a variety of heterostructure nanomaterials to be synthesized.

CdE nanorod growth can be promoted by inducing a burst of particle nucleation and then adding more reactant at low supersaturation to alleviate further particle nucleation and favor epitaxial deposition on the{002}surfaces,which appear to the most reactive facet of the nanocrystal/nanorod.These findings of face-sensitive reactivity are consistent with recent observa-tions in the case of Cu2S nanodisks27and Bi2S3nanowires,28in which anisotropic growth is promoted due to enhanced“mono-mer”epitaxy on particular facets.It is well-known that thin film epitaxial growth rates in gas-phase deposition methods depend sensitively on the exposed crystal plane of the substrate.We have shown here that anisotropic face-sensitive epitaxial deposi-tion can occur on colloidal semiconductor surfaces in solution. The next step is to ascertain the potential to extend epitaxial selectivity to other materials,including those with isotropic crystal structure.The tetrapod formation observed by Alivisatos et al.in ref15provides encouraging evidence that epitaxial selectivity can be promoted in these materials as well. Acknowledgment.This work is supported in part by the Welch Foundation,the STC Program of the National Science Foundation under agreement number CHE-9876674,and the Advanced Materials Research Center(AMRC)in collaboration with International SEMATECH.

Supporting Information Available:Description and details of nanocrystal,nanorod and heterostructure synthesis and characterization.This material is available free of charge via the Internet at https://www.sodocs.net/doc/d82470341.html,.

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歌舞剧 猫 中英对照歌词

Are you blind when you're born? Can you see in the dark? 你出生时是目盲的吗？你能在黑暗处看到事物吗？ Dare you look at a king? Would you sit on his throne? 你敢目室国王吗？你想坐在王位上吗？ Can you say of your bite that it's worse than your bark? 你能说你的咬力不如你的叫声吗？ Are you cock of the walk when you're walking alone? 当你独自行走时你很自信自傲吗？ Because jellicles are and jellicles do 因为杰利克是杰利克能 Jellicles do and jellicles would 杰利克能杰利克会 Jellicles would and jellicles can 杰利克会杰利克能 Jellicles can and jellicles do 杰利克能杰利克做 When you fall on your head, do you land on your feet? 当你头朝下落下时，你能用脚着地吗？ Are you tense when you sense there's a storm in the air? 当你感到风暴来临时，你会很紧张吗？ Can you find your way blind when you're lost in the street? 当你迷路时，你能本能的找到正确的方向吗？ Do you know how to go to the heaviside layer? 你知道如何升向九重天吗？ Because jellicles can and jellicles do 因为杰利克能杰利克做 Jellicles do and jellicles can 杰利克做杰利克能 Jellicles can and jellicles do 杰利克能杰利克做 Jellicles do and jellicles can 杰利克做杰利克能 Jellicles can and jellicles do 杰利克能杰利克做 Can you ride on a broomstick to places far distant? 你能骑着扫把去很远的地方吗？ Familiar with candle, with book, and with bell? 你喜爱玩耍蜡烛，书籍或是铃铛吗？ Were you Whittington's friend? The Pied Piper's assistant? 你是惠廷顿的朋友？或是吹笛手的助理吗？ Have you been an alumnus of heaven and hell? 你能自由的通往天堂和地狱吗？ Are you mean like a minx? Are you lean like a lynx? 你是一个爱出风头的姑娘吗？你瘦的像一只山猫吗？ Are you keen to be seen when you're smelling a rat? 当你闻到一只老鼠你会努力的寻找吗？ Were you there when the pharaoh commissioned the Sphinx? 当法老委派做狮身人面像时你在场吗？ If you were, and you are, you're a jellicle cat 如果你在并且你是，你是一只杰利克猫． Jellicle songs for jellicle cats 杰利克歌咏杰利克猫 Jellicle songs for jellicle cats 杰利克歌咏杰利克猫 Jellicle songs for jellicle cats 杰利克歌咏杰利克猫

歌词

我的歌声里 没有一点点防备 也没有一丝顾虑 你就这样出现 在我的世界里带给我惊喜情不自己可是你偏又这样 在我不知不觉中悄悄地消失 从我的世界里没有音讯 剩下的只是回忆 你存在我深深的脑海里 我的梦里我的心里我的歌声里 你存在我深深的脑海里 我的梦里我的心里我的歌声里 还记得我们曾经 肩并肩一起走过那段繁花巷口 尽管你我是陌生人是过路人 但彼此还是感觉到了 对方的一个眼神一个心跳 一种意想不到的快乐 好像是一场梦境命中注定 你存在我深深的脑海里 我的梦里我的心里我的歌声里 你存在我深深的脑海里 我的梦里我的心里我的歌声里 世界之大为何我们相遇 难道是缘分难道是天意 你存在我深深的脑海里 我的梦里我的心里我的歌声里 你存在我深深的脑海里 我的梦里我的心里我的歌声里 你存在我深深的脑海里 我的梦里我的心里我的歌声里 如水 期待过我们似细水 可惜蒸发出眼泪 明白你最近有些暂时伴侣偷一刻午睡彷佛专一使你极空虚 怀疑被你抱着我念着谁 无论你再好亦舍得失去 难过亦过难道我 嫌损失未够多

早放手可减轻痛楚 不等泡沫给吹破 不想去知谁填补我 无悔在我还是我 任你多么差错 无谓去追问为何 深知告别损失非我 让情人离别 似水清洗我 原谅你对着我说谎 出于好意的作状 明白你最近已经避谈近况 早不敢寄望 心中早把相爱如观光 情如瀑布泻下也未惊慌 心境已随着那水花得到释放 难过亦过难道我 嫌损失未够多 早放手可减轻痛楚 不等泡沫给吹破 不想去知谁填补我 无悔在我还是我 任你多么差错 无谓去追问为何 深知告别损失非我 让情人离别 似水清洗我 难过亦过难道我 嫌损失未够多 早放手可减轻痛楚 不等泡沫给吹破 不想去知谁填补我 无悔在我还是我 任你多么差错 无谓去追问为何 深知告别损失非我 让情人离别 似水清洗我 心中有涟漪吹过又回到最初平静去做我

英语文化 学英语必须要知道的经典英文歌曲14 Hallelujah

歌曲背景 "Hallelujah" is a song written by Canadian singer Leonard Cohen, originally released on his album Various Positions (1984). Achieving little initial success, the song found greater popular acclaim through a recording by John Cale, which inspired a recording by Jeff Buckley. It has been viewed as a "baseline" for secular hymns. "Hallelujah"为加拿大著名游吟诗人、民谣歌手Leonard Cohen在1985年创作的歌曲，收录在其专辑"Various Positions"中。其歌词充满诗意，内涵丰富，曲调缓慢忧伤，加上Leonard沧桑嗓音的低吟浅唱，演绎出了一种清淡而悠长的回味。 Hallelujah的版本很多，其中最有影响力的还是美国著名创作型歌手Jeff Buckley的翻唱版本，被收录在其1994年的专辑"Grace"中。Jeff被U2的Bono形容为“噪海中的纯净一滴”，他的声音明丽甜蜜又性感飘渺，诠释起悲伤和记忆来却更令人印象深刻。 中国歌手邓紫棋在现场演唱会上翻唱了本曲。 英文歌词 Now I've heard there was a secret chord 我曾听闻一曲传奇中的旋律 That David played, and it pleased the Lord 是大卫弹奏来取悦上帝的赞颂 But You don't really care for music, do You? 但祢真正喜悦的(是人的作为，而)不是音乐，对吧？ Well it goes like this 旋律是这样的 The fourth, the fifth F和弦，G和弦(复杂的心情无可言喻) The minor fall, the major lift 大小调起承转合(指戴维泣不成声的祷告颂唱，至五音不全) The baffled king composing Hallelujah

英文典范歌谣一起唱1A1B1C歌词

1A 1.Are You Sleeping? Are you sleeping? Are you sleeping? Brother John, Brother John? Morning bells are ringing, Morning bells are ringing. Ding, ding, dong! Ding, ding, dong! 2.Ten Little Indians One little, two little, three little Indians,

Four little, five little, six little Indians, Seven little, Eight little, Nine little Indians, Ten little Indian boys. One little, two little, three little Indians, Four little, five little, six little Indians, Seven little, Eight little, Nine little Indians, Ten little Indian girls. 3.Happy Birthday to You Happy birthday to you. Happy birthday to you. Happy birthday, dear friend. Happy birthday to you.

4.Hot Potato One potato, two potatoes, Three potatoes, four, Five potato, six potatoes, Seven potatoes, more. 5.Hot Cross Buns Hot cross buns! Hot cross buns! One a penny, two a penny. Hot cross buns! If you have no daughters, Give them to you sons!

English song-as long as you love me英文经典脍炙人口歌曲歌词解析

歌名：As Long As You Love Me 歌手：Justin Bieber 所属专辑：Believe Acoustic 作曲 : Persson Svensson 作词 : Persson Svensson As long as you love me yeah 只要你爱我就好 I'm under pressure, seven billion people in the world trying to fit in 我们在压力下跟着全世界70亿人适应这个社会 Keep it together, smile on your face even though your heart is frowning 紧紧相依，你心有困懑却面带笑容 But hey now, you know girl, we both know it's a cruel world 但是现在，宝贝你知道，我们都知道世界多么残酷 But I will take my chances 但我愿意（搏一搏）抓住我的机会 As long as you love me, we could be starving, 只要你爱我，我们可以挨饿（饥肠辘辘） We could be homeless, we could be broke 可以流离失所，也可以支离破碎 As long as you love me I'll be your platinum, I'll be your silver, i'll be your gold 只要你爱我，我是你的铂金，我是你的银，我是你的财富（我会不离不弃，无坚不摧，所向披靡）

英文歌词

1、《Mister Sun》 Oh Mister Sun, Sun, Mister Golden Sun, Please shine down on me. Oh Mister Sun, Sun,Mister Golden Sun, Hiding behind a tree… These little children ， Are asking you To please come out So we can play with you. Oh Mister Sun, Sun,Mister Golden Sun, Please shine down on me! Oh Mister Sun, Sun, Mister Golden Sun, Please shine down on me. Oh Mister Sun, Sun, Mister Golden Sun,Hiding behind a tree…These little children Are asking youTo please come out So we can play with you. Oh Mister Sun, Sun,Mister Golden Sun, Please shine down on,Please shine down on, Please shine down on me! 2、Mango Walk My brother did a tell me That you go mango walk You go mango walk(2×) My brother did a tell me That you go mango walk And pick all the numbe r ?leven 3、Mosquito Mosquito one, Mosquito two. Mosquito jump in the old man ,shoe Zzzzzzzz(clap the mosquito ) 4、Artist：harrybelafonte Songs Title：coconut woman （Coconuts, coconuts） （Coconuts, coconuts） Coconut woman is calling out And everyday you can hear her shout Coconut woman is calling out And everyday you can hear her shout Get your coconut water （Four for five） Man, it's good for your daughter （Four for five） Coco got a lotta iron （Four for five） Make you strong like a lion （Four for five） A lady tell me the other day No one can take her sweet man away I ask her what was the mystery She say coconut water and rice curry You can cook it in a pot （Four for five） You can serve it very hot （Four for five） Coco got a lotta iron （Four for five） Make you strong like a lion （Coconuts, coconuts） Coconut woman says you'll agree Coconut make very nice candy The thing that's best If you're feeling glum Is coconut water with a little rum It could make you very tipsy （Four for five） Make you feel like a gypsy （Four for five） Coco got a lotta iron （Four for five） Make you strong like a lion （Four for five） Ah, play that thing Coconut woman is calling out And everyday you can hear her shout Coconut woman is calling out And everyday you can hear her shout Get your coconut water （Four for five） Man, it's good for your daughter （Four for five） Get your coconut candy （Four for five） Make you feel very dandy （Four for five） Coco, coco, coco... Coconut, coconut Coconut, coconut... -

听的圣诞节英语歌曲

听的圣诞节英语歌曲 下面是一些圣诞节英文歌曲推荐！ 1、Everybody Knows I Love U 圣诞表白 2、Hallelujah-Alexandra Burke圣诞单曲销售冠军 3、圣诞必听英文歌曲John Lennon(Happy Christmas) 4、豌豆公主Kylie Minogue圣诞情调Santa Baby 5、小天后Taylor Swift演绎缤纷圣诞Last Christmas 6、NIKE最新圣诞广告歌曲完整版 7、Lady GaGa 欢乐圣诞单曲Christmas Tree 8、最畅销圣诞歌Mariah Carey(All I Want For Christmas Is You) 9、超人气童星Justin Bieber在奥巴马总统面前献唱圣诞歌曲 10、可爱童声贺圣诞When Christmas comes to town 欢乐合唱团相约快乐圣诞 Glee Cast - Last Christmas 美国福克斯电视台于2009年推出的热门青春音乐剧《欢乐合唱团》Glee盛邀剧中的男女主演们，包括Lea Michele, Amber Riley, Cory Monteith, Kevin McHale, Jenna Ushkowitz, Chris Colfer, Dianna Agron, Mark Salling等一席欢乐合唱团的团员们齐齐出动，为我们带来了这首欢快的经典翻唱"Last Christmas"。 绯闻女孩Queen B喊你回家过圣诞 Leighton Meester - Christmas "Christmas (Baby Please Come Home)"是Darlene Love于1963年发表的经典圣诞歌曲，后被乐队U2、乐坛天后Mariah Carey翻唱。

hallelujah英文歌词

I've heard there was a secret chord That David played, and it pleased the Lord But you don't really care for music, do you? It goes like this The fourth, the fifth The minor fall, the major lift The baffled king composing Hallelujah Hallelujah, Hallelujah Hallelujah, Hallelujah Your faith was strong but you needed proof You saw her bathing on the roof Her beauty in the moonlight overthrew you She tied you to a kitchen chair She broke your throne, and she cut your hair And from your lips she drew the Hallelujah Hallelujah, Hallelujah Hallelujah, Hallelujah Baby I have been here before I know this room, I've walked this floor I used to live alone before I knew you. I've seen your flag on the marble arch Love is not a victory march It's a cold and it's a broken Hallelujah Hallelujah, Hallelujah Hallelujah, Hallelujah Maybe there’s a God above But all I’ve ever learned from love Was how to shoot at someone who outdrew you It’s not a cry you can hear at night It’s not somebody who has seen the light It’s a cold and it’s a broken Hallelujah Hallelujah, Hallelujah Hallelujah, Hallelujah I did my best, it wasn't much I couldn't feel, so I tried to touch I've told the truth, I didn't come to fool you And even though it all went wrong I'll stand before the Lord of Song With nothing on my tongue but Hallelujah

英文歌歌词

Miley Cyrus - The Climb / 麦莉·赛勒斯- 攀登 I can almost see it / 眼前依稀浮现 That dream I'm dreamin' but / 萦绕心头的那个梦境There's a voice inside my head saying / 脑海里却响起一个声音 you'll never reach it / 你永远也不会到达彼岸Every step I'm taking / 我迈出的每一步 Every move I make feels /我做过的每件事 Lost with no direction / 无不使我迷失方向 My faith is shakin / 开始动摇的，是我的信念 But I, I gotta keep tryin. / 可我，我还是要继续求索Gotta keep my head held high / 还是要挺胸抬头、阔步前行 There's always gonna be another mountain / 总会有下一座山峦 I'm always gonna wanna make it move / 在等我去将它移开 Always gonna be an uphill battle / 总会有下一个山坡 Sometimes I'm gonna have to lose / 很可能令我无法越过 Ain't about how fast I get there / 不在于我要用多久才能抵达峰顶 Ain't about what's waitin on the other side / 不在于山那边倒底是怎样的风景 It's the climb / 这就是攀登 The struggles I'm facing / 我面对的每次搏击 The chances I'm taking / 我抓住的每次机遇Sometimes might knock me down but / 有时会令我一败涂地 No I'm not breaking / 却决不会磨去我的意志 I may not know it / 或许我不懂其中的意义 But these are the moments that / 但这些时刻却会成为 I'm gonna remember most, yeah / 我一辈子可以珍藏的回忆，啊 Just gotta keep going / 只管继续前进 And I, I gotta be strong / 我要，我要变得坚强 Just keep pushing on 'cause / 只须奋力前行，因为 There's always gonna be another mountain / 总会有下一座山峦I'm always gonna wanna make it move / 在等我去将它移开 Always gonna be an uphill battle / 总会有下一个山坡 Sometimes I'm gonna have to lose / 很可能令我无法越过 Ain't about how fast I get there / 不在于我要用多久才能抵达顶峰 Ain't about what's waitin on the other side / 不在于山那边倒底是怎样的风景 It's the climb / 这就是攀登 Yeah-yeah / 啊- There's always gonna be another mountain / 总会有下一座山峦 I'm always gonna wanna make it move / 在等我去将它移开 Always gonna be an uphill battle / 总会有下一个山坡 Sometimes you're gonna have to lose / 很可能令我无法越过 Ain't about how fast I get there / 不在于我要用多久才能抵达顶峰 Ain't about what's waitin on the other side / 不在于山那边倒底是怎样的风景 It's the climb / 这就是攀登 Yeah-yeah-yeah / 啊- - Keep on moving / 继续前行 Keep climbing / 继续攀登 Keep the faith / 坚守信念 Baby / 宝贝 It's all about / 这一切就是 It's all about the climb / 这一切就是攀登

Alexandra Burke - Hallelujah

Hallelujah Well I heard there was a secret chord 我听说有个神秘的和弦 That David played, and it pleased the Lord 大卫弹奏以取悦主 But you don't really care for music, do ya? 可你并不关心音乐，不是么 Well it goes like this 它这样奏起 The fourth, the fifth 四度，五度(2)

The minor fall and the major lift 小调降，大调升The baffled king composing Hallelujah 徒然哀求的君王谱下哈利路亚(3) Hallelujah Hallelujah 哈利路亚哈利路亚 Hallelujah Hallelujah 哈利路亚哈利路亚Well Your faith was strong but you needed proof 你信心坚定但需受考验 You saw her bathing on the roof 你在屋顶见她沐浴 Her beauty and the moonlight overthrew you 她在月光下的美丽将你击溃(4) She tied you to her kitchen chair 她将你捆在厨房的椅上 And she broke your throne and she cut your hair 她毁了你的王位剪下你的头发(5) And from your lips she drew the Hallelujah 从你的唇中她吸吮哈利路亚 Hallelujah Hallelujah 哈利路亚哈利路亚 Hallelujah Hallelujah 哈利路亚哈利路亚

Rufus Wainwright - Hallelujah中英文歌词对照(伤感抒情英文)

Rufus Wainwright - Hallelujah 歌词翻译： I heard there was a secret chord that David played and it pleased the Lord But you don’t really care for music, do you? Well it goes like this : The fourth, the fifth, the minor fall and the major lift The baffled king composing Hallelujah 我听见了那神秘悠扬的旋律 那是以色列王（David）为取悦上帝而奏 但也许你并不在意旋律本身，不是吗？ 音乐却是这样起来的 第4，第5，小调落下，大调升起 饱受煎熬的国王写下了赞美之歌－哈利路亚 Hallelujah Hallelujah Hallelujah Hallelujah… 哈利路亚，哈利路亚，哈利路亚““` Your faith was strong but you needed proof You saw her bathing on the roof Her beauty and the moonlight overthrew you And she tied you to her kitchen chair She broke your throne and she cut your hair But from your lips she drew the Hallelujah 你信念坚定却也要受到考验 你在屋顶上看到她在那里沐浴 她的美貌在月光下就已经把你征服 她会把你骗到坐上厨房里的椅子上 推翻你的宝座，并剪下你的发丝 为了听到你的唇边的赞美之歌－哈利路亚 Hallelujah Hallelujah Hallelujah Hallelujah… 哈利路亚，哈利路亚，哈利路亚“““` Baby I’ve been here before I’ve seen this room and I’ve walked this floor I used to live alone before I knew ya And I’ve seen your flag on the marble arch

70首唯美欧美歌推荐

Turn off the Lights 70首唯美欧美歌推荐 Ruolin_run 很久没有写文了，近来无事，方生一念，将库存里的歌整一整，分了类，挑出这70首唯美曲。先说明，这70首曲风绝对是极唯美的，绝大多数属于英文民谣或蓝调，有部分是小众派，大多数以钢琴、吉他伴奏，先后顺序无优劣之分，请关上灯，戴上耳机，不要受打扰，自己一个人听。 噢…再说一句，你看我打了这么多，路过的，请留贴 1.30 Minutes-T.A.T.U 曾经风靡一时的俄罗斯少女二重唱组合为我们带来的纯唱…你一定会爱上的…好像夜空中划过的流星..歌曲以音乐的笑声开场，带出旋律，伴奏不显眼，最后全曲又不知不觉消失… 2.A Perfecr Indian-Sinead O’Connor 全曲以钢琴伴奏开场，你听懂了歌手的吟语吗…她唱出了一种独特的孤独…一个年轻就剃光头的女子必是孤独的… 3.A Place Nearby-Lene Marlin 挪威小才女Lene Marlin的代表作，轻轻哼唱，没有震撼感，就像你的邻家小女孩的哼唱一样，但绝对能攫住你的心 4.Black Star-Avril Lavigne 歌手绝对是众所周知的了，但歌曲却不怎么著名…这是Avril歌中最抒情的一首之一，以近似八音盒的乐器开场，清脆，悠扬… 5.Bluebird-Christina Perri 我居然把我最喜欢的歌手排到第五…全曲基本以吉他为主旋律伴奏，曲调轻快悠扬，富有生机…歌手是民谣歌手，目前不著名，但是底子很厚，但民谣歌手的身份，让她不容易红起来… 6.Breathe Me-Sia 歌手声音稍稍沙哑，呓语恰与钢琴伴奏的欢快明亮形成了对比，别有独特的滋味… 7.Butterfly Fly Away-Miley Cyrus 这个肯定很多人听过啦…类似于吉他的自弹自唱，高潮部分的父女双声部合唱更是感人，是一个少女对未来的憧憬… 8.By Our Love-Christy Nockels 这其实是宗教歌曲，但如果你没查歌词…是看不出来的，曲风庄严唯美，感人至深…舒缓的钢琴旋律配合着歌手醇厚的嗓音，缓缓淌出…听一遍，就会被迷住… 9. Caresse Sur L'Ocean-Kelly Sweet 这首《放牛班的春天》的主题曲，经过甜心Kelly的演绎，褪去了少年的青涩，变得更为纯美，同样空灵澄澈… 10.Childhood-Michael Jackson 歌手太著名，致敬…唱出了一个唯美的理想儿童世界，MV中的Michael却一人独自流出感伤之情，是对自己的童年的感伤么…曲风唯美感伤，Michael声音中的空灵发挥到了极致，全曲有电影艺术的感觉… 11．Come Away With Me-Norah Jones 这个歌手也太著名…爵士才女，这是她的代表作，很能体现她像葡萄酒冰激凌一样醇厚的嗓音… 12.Corner of Your Heart-Ingrid Michaelson 与前面的A Perfect Heart曲风相似，都有种不经意间的孤独之感…女声空旷灵澈，属于多听几遍才会爱上的类型… 13.Craigie Hill-Cara Dillon

Hallelujah(帮你更好理解这首歌)

《Hallelujah》背后的故事： Hallelujah，哈利路亚，希伯来语，意为“赞美上帝”。邓紫棋演唱的这首《Hallelujah》，是加拿大著名诗人/作家/歌手Leonard Cohen，在1984年的专辑《Various Positions》中那首最为著名的同名单曲。 《Hallelujah》歌词几乎是处处依托圣经故事的。比如在第一段歌词中提到的David。David，大卫，牧羊人出身，但容貌俊美，英勇善战，能赋能歌，战胜巨人哥利亚，被上帝选为以色列的国王。在大卫当国王的时候，一日傍晚，在阳台闲逛时偶然发现一貌美女子正在沐浴（《Hallelujah》歌词中的You saw her bathing on the roof / Her beauty and the moonlight overthrew you），娇媚性感的曲线加上柔和迷人的月光将大卫彻底吸引住。之后，大卫便派人四处打听此女子，想要知道她的芳名。原来，这个迷人的女子名叫Bethsheba （拔示巴），是大卫的一位部将Uriah（乌利亚）的妻子。大卫忍受不住占有拔示巴的欲望，终于让人将拔示巴接入宫中，与其同房。不久，拔示巴怀上了大卫的孩子，大卫恐慌万分，急忙召回远在前线的乌利亚，借口让其休整一下，意图让乌利亚回到家中与妻子同房以掩盖拔示巴肚中孩子的亲缘归属。 但是，乌利亚是一位忠于职守为国尽忠的勇士，他对大卫说：“国家处于危机，我怎有心思回家与妻子相欢，溺于安享。”乌利亚要求大卫将自己重新派回到战场上。大卫此时便顺水推舟，并写成密信一封，让乌利亚携信到大将军约亚那里；信中大卫指示约亚将乌利亚派往最为危险的战场。于是，乌利亚就在大卫的密谋和意愿下战死沙场，而大卫则将拔示巴迎进自己的后宫，名正言顺的占有了拔示巴。 然而，占有拔示巴的大卫并不快乐，他白天对着众人强颜欢笑，夜晚就成为自己罪过的奴隶，受尽折磨。大卫认识到自己的罪行，写下诗篇五十一篇忏悔书，歌与上帝，祈求宽恕（Now I've heard there was a secret chord / That David played, and it pleased the Lord / But you don't really care for music, do you?） “She tied you T o a kitchen chair / She broke your throne, and she cut your hair” 这个场景则是Samson（参孙）和Delilah（达利拉）的故事。以色列在被非力士人统治的时候，族中有个大力士，名叫参孙，上帝赐予他空手撕裂雄狮的神力，这使得非力士统治者颇为惧怕，但是，参孙有个弱点：上帝与其约定——不得剪发，如是，则神力尽失。参孙爱上了一位非力士族的姑娘，名叫达利拉。非力士统治者赐予达利拉许多钱财，命令她与参孙相好并套出他为何力大无穷的秘密。参孙在达利拉的三次诱惑下以编造的故事将其蒙混，但是最后参孙还是将自己的秘密告诉的达利拉。一日，达利拉趁安抚参孙熟睡于自己的膝上时，让人将参孙的头发剪掉了。参孙醒来，发现自己的头发被剪，神力也一并消失了。可怜的参孙在爱情的迷惑下，违背了与神定下的誓言，从一个英勇的大力士变成了一个人人欺辱的瞎子。这首歌的歌词里，也描写了作为罪人在罪恶中的迷茫、迷惘和空虚失落；被罪恶所辖制的痛苦；而要要从罪中结果，脱离罪的辖制，惟有借着主耶稣宝贵血的恩典才可以做到；也许这正是邓紫棋在那见证中所经历的过程；但你重回主耶稣的怀抱中时，一切的不安、迷惘、空虚都离你而去了，从此你得到满足。 那时，你就会情不自禁的开口赞美主，如作者Leonard Cohen所说，“当一个人展望世界回首生命时，唯一可言的词语便是Hallelujah”。 创作信息 "Hallelujah"为加拿大著名游吟诗人、民谣歌手Leonard Cohen在1985年创作的歌曲，收录在其专辑"Various Positions"中。其歌词充满诗意，内涵丰富，曲调缓慢忧伤，加上Leonard 沧桑嗓音的低吟浅唱，演绎出了一种清淡而悠长的回味。 Jeff Buckley翻唱版本

Hallelujah中英文歌词

hallelujah I heard there was a secret chord 我听见了那神秘悠扬的旋律 that David played and it pleased the Lord 那是以色列王（David）为取悦上帝而奏 But you don't really care for music, do you? 但也许你并不在意旋律本身，不是吗？ Well it goes like this : 音乐却是这样起来的 The fourth, the fifth, the minor fall and the major lift 第4，第5，小调落下，大调升起 The baffled king composing Hallelujah 饱受煎熬的国王写下了赞美之歌－哈利路亚 Hallelujah HallelujahHallelujahHallelujah... 哈利路亚，哈利路亚，哈利路亚````` Your faith was strong but you needed proof 你信念坚定却也要受到考验 You saw her bathing on the roof 你在屋顶上看到她在那里沐浴 Her beauty and the moonlight overthrew you 她的美貌在月光下就已经把你征服 And she tied you to her kitchen chair 她会把你骗到坐上厨房里的椅子上 She broke your throne and she cut your hair 推翻你的宝座，并剪下你的发丝 But from your lips she drew the Hallelujah 为了听到你的唇边的赞美之歌－哈利路亚 Hallelujah HallelujahHallelujahHallelujah... 哈利路亚，哈利路亚，哈利路亚``` ````

ハレルヤ(哈利路亚)rurutia 歌词

ハレルヤ（哈利路亚） 专辑：Promised Land 歌手：RURUTIA （ルルティア） 作词：RURUTIA （ルルティア） 作曲：RURUTIA （ルルティア） 翻译：风之阡陌 远くこだまするは獣たち/ 远处传来的声音是野兽们 深い夜に罪を笑い语る/ 在深夜里狞笑着谈论罪行 血涂られた正义/ 血染的正义 汚れた身体を/ 污秽的身体 锖びた雨が磨く/ 被生锈的雨水刷洗 重ねた过ちた饰られた街に/ 装饰着重复罪过的街道上 死の灰が降る/ 死之灰烬降下 甘く忍びよるは魔物たち/ 天真潜近的妖魔们 穴の开いた胸に笑いかける/ 朝着打开的胸口冷笑 堕落する天使/ 堕落的天使 圣なる翼と替えた/ 与圣洁羽翼交换的 禁断の杯/ 禁忌之杯 涡巻く欲望は加速した/ 被加速卷起漩涡的欲望 街は沈んでいく/ 渐渐地沉没在街道上 OH ハレルヤ全て洗い流して/ OH 哈利路亚将一切冲洗吧

汚れた身体を/ 污秽的身体 锖びた雨が磨く/ 被生锈的雨水刷洗 重ねた过ちた饰られた街に/ 装饰着重复罪过的街道上死の灰が降る/ 死之灰烬降下 圣なる翼と替えた/ 与圣洁羽翼交换的 禁断の杯/ 禁忌之杯 涡巻く欲望は加速して/ 被加速卷起漩涡的欲望 街は沈んでいく/ 渐渐地沉没在街道上 汚れた身体を/ 污秽的身体 锖びた雨が磨く/ 被生锈的雨水刷洗 重ねた过ちた饰られた街に/ 装饰着重复罪过的街道上死の灰が降る/ 死之灰烬降下 to o ku ko da ma su ru wa ke mo no ta chi fu ka ku yo ru ni tsu mi wo wa ra i ka ta ru chi nu ra re ta se i gi yo go re ta ka ra da wo sa bi ta a me ga mi ga ku ka sa ne ta a ya ma chi de ka za ra re ta ma chi ni shi no ha i ga fu ru a ma ku shi no bi yo ru wa ma mo no ta chi a na no a i ta mu ne ni wa ra i ka ke ru

最经典的五首英文歌曲

最经典的五首英文歌曲 不仅旋律优美动听，而且歌词可读性高。1．only love Two a m and the rain is falling Here we are at the crossroads once again You're telling me you're so confused You can't make up your mind Is this meant to be You're asking me But only love can say Try again or walk away But I believe for you and me The sun will shine one day So I just play my part Pray you'll have a change of heart But I can make you see it through That's something only love can do In your arms as the dawn is breaking Face to face and a thousand miles apart I've tried my best to make you see There's hope beyond the pain If we give enough If we learn to trust

But only love can say Try again or walk away But I believe for you and me The sun will shine one day So I just play my part Pray you'll have a change of heart But I can make you see it through That's something only love can do I know if I could find the words To touch you deep inside You'll give my dreams just one more chance To let this be our last goodbye But only love can say Try again or walk away But I believe for you and me The sun will shine one day So I just play my part Pray you'll have a change of heart But I can make you see it through That's something only love can do That's something only love can do